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oapen-20.500.12657-868502024-01-15T17:31:13Z Dynamic Model-based Analysis of Oxygen Reduction Reaction in Gas Diffusion Electrodes Röhe, Maximilian Chlor-alkali electrolysis; Three-phase model; Electrochemical Mass Spectroscopy; Inhomogeneous electrode structure; Chloralkali-Elektrolyse; Dreiphasen Modellierung; Elektrochemische Massenspektroskopie; Maxwell-Stefan Diffusion; Inhomogene Elektrodenstruktur bic Book Industry Communication::T Technology, engineering, agriculture::TH Energy technology & engineering::THR Electrical engineering In this work, the first simulation model of oxygen depolarized cathodes (ODC), which are silver catalyst-based gas diffusion electrodes, is presented that considers the phase equilibrium of the gas-liquid interface and structure-related inhomogeneities in electrolyte distribution. By means of the model it has been identified that mass transport of water and ions in the liquid phase is a crucial factor for electrode performance and how it is influenced by the electrode structure. 2024-01-15T13:10:04Z 2024-01-15T13:10:04Z 2024 book https://library.oapen.org/handle/20.500.12657/86850 eng Schriftenreihe des Instituts für Angewandte Materialien, Karlsruher Institut für Technologie application/pdf Attribution 4.0 International dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf https://doi.org/10.5445/KSP/1000150805 KIT Scientific Publishing 10.5445/KSP/1000150805 10.5445/KSP/1000150805 44e29711-8d53-496b-85cc-3d10c9469be9 109 178 open access
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OAPEN
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English
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description |
In this work, the first simulation model of oxygen depolarized cathodes (ODC), which are silver catalyst-based gas diffusion electrodes, is presented that considers the phase equilibrium of the gas-liquid interface and structure-related inhomogeneities in electrolyte distribution. By means of the model it has been identified that mass transport of water and ions in the liquid phase is a crucial factor for electrode performance and how it is influenced by the electrode structure.
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title |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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spellingShingle |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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title_short |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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title_full |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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title_fullStr |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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title_full_unstemmed |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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title_sort |
dynamic-model-based-analysis-of-oxygen-reduction-reaction-in-gas-diffusion-electrodes.pdf
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publisher |
KIT Scientific Publishing
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publishDate |
2024
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url |
https://doi.org/10.5445/KSP/1000150805
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1799945302170402816
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